Actually, that was exactly the idea I had in mind when I first thought of it. Not right now, she can't, but eventually she will. It requires absolute concentration, and it's difficult for even a badass like Charlotte to achieve it right yet. Plus, the body of the enemy tends to move alot, so Charlotte will have difficulty grabbing the dude's heart and yanking it out even when she and Chibi-Phantomere achieve a strong level of trust and experience.
More than likely, she'll find it more useful to have Chibi-Phantomere possess things. Chibi-Phantomere could make thrown objects deal more damage by possessing them and arching them around to hit weaker areas. He can also do more obscure things, like say, make a gatling gun misfire by possessing the gun and causing the rotating barrels to halt. It's like a severely downscaled version of Matthias's hacking abilities.
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